Cannot send emails

I have tiscali email accounts that have worked fine until yesterday (18/1/16). Now every send fails with
- Sending' reported error (0x800CCC6F) : 'Your outgoing (SMTP) e-mail server has reported an internal error. If you continue to receive this message, contact your server administrator or Internet service provider (ISP). The server responded: 554 cm12gb1 smtp.talktalk.net LeIiavvMEy4wx Bad IP Reputation (TT101)